It seems that you have several network problems, the VAMi on the 5480 (of the old vCenter) is crucial to be able to transfer the data and start the vcsa services correctly, I advise you to delete the new vCenter and start over with the depèloyment procedure (make sure before you can reach everything inside the network)
furthermore, if your old vcenter is still OK, I suggest you, as usual, make a backup from VAMI and, for safety, also make a clone of it before starting again